Radiation intensity of lignite-fired oxy-fuel flames

• The radiative heat transfer in oxy-fuel flames is compared to corresponding conditions in air-fuel flames during combustion of lignite in the Chalmers 100 kW oxy-fuel test facility. In the oxy-fuel cases the flue-gas recycle rate was varied, so that, in principle, the same stoichiometry was kept in all cases, whereas the oxygen fraction in the recycled flue-gas mixture ranged from 25 to 29 vol.%. Radial profiles of gas concentration, temperature and total radiation intensity were measured in the furnace. The temperature, and thereby the total radiation intensity of the oxy-fuel flames, increases with decreasing flue-gas recycle rate. The ratio of gas and total radiation intensities increases under oxy-fuel conditions compared to air-firing. However, when radiation overlap between gas and particles is considered the ratios for air-firing and oxy-fuel conditions become more similar, since the gas-particle overlap is increased in the CO2-rich atmosphere. A large fraction of the radiation in these lignite flames is emitted by particles whose radiation was not significantly influenced by oxy-fuel operation. Therefore, an increment of gas radiation due to higher CO2 concentration is not evident because of the background of particle radiation, and, the total radiation intensities are similar during oxy-fuel and air-fuel operation as long as the temperature distributions are similar.

Ämnesord

NATURVETENSKAP  -- Kemi -- Annan kemi (hsv//swe)

NATURAL SCIENCES  -- Chemical Sciences -- Other Chemistry Topics (hsv//eng)

Nyckelord

Gas radiation

Combustion

Heat transfer

CO2 reduction

Oxy-fuel

Particle radiation

Publikations- och innehållstyp

art (ämneskategori)

ref (ämneskategori)